Dr. Marin Alexe
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Original publication

Daniel Pantel, Silvana Goetze, Dietrich Hesse und Marin Alexe
Reversible electrical switching of spin polarization in multiferroic tunnel junctions

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A filter for electron spins

Diagram of a multiferroic material sandwich: The orange-red base carries a green layer of ferromagnetic lanthanum strontium manganate (LSMO). Above th Zoom Image
Diagram of a multiferroic material sandwich: The orange-red base carries a green layer of ferromagnetic lanthanum strontium manganate (LSMO). Above that is the insulating ferroelectric lead zirconate titanite (PZT) layer. The nano condensers are completed by ferromagnetic cobalt electrodes. They get their shape from correspondingly structured shadow masks. In reality, the PZT layer is considerably thinner than the LSMO layer; it is barely three nanometres thick. [less]

The physicists in Halle actually observed the normal tunnel magnetoresistance in one of the two electric polarisation directions in the ferroelectric PZT layer. In the case of the other electric polarisation direction, however, reverse conditions surprisingly occurred – now there was inverted TMR. The tunnel connection conducts current with little resistance when the two ferromagnets are magnetised in the opposite direction.

Apart from the effect on the electric resistance, the TMR also acts as an electron spin filter. In simple terms, the spin is the direction in which the electrons are spinning; it provides every electron with its own magnetic momentum, which may point into one or the other direction. In the simplest case of normal TMR, only electrons whose magnetic momentum is pointing in the same direction as the magnetisation of the two ferromagnetic electrodes manage to get through the PZT layer. “A change in the electric polarisation direction therefore influences the strength of the tunnel current and also results in electrons with a certain spin being filtered out,” explains Marin Alexe. “We can achieve the same effect by changing the magnetisation in both ferromagnetic layers with an external magnetic field, but this method uses a lot more energy.”

The influence of the electric polarisation on the filter effect of the tunnel junction for electron spins and the electric resistance are interesting for applications, because, all in all, the multiferroic tunnel junction can take four different values of the electric resistance: two for each electric polarisation direction, one for the same magnetisation and one for opposite magnetisation of the two ferromagnets. “This enables us to deposit three times as much information in a multiferroic tunnel junction than in ordinary binary magnetic storage,” comments Marin Alexe. This means that the size of magnetic random access memories (MRAM) can be considerably reduced. MRAMs provide an alternative to conventional electrically operated RAMs. They would make it unnecessary to load data from the hard drive to the main working memory when booting up a computer, and the device would be ready to use at the push of a button.

Better understanding to pave the way for spintronics

“As a filter that can be simply switched and sort electrons according to their spin direction, the multiferroic tunnel junction could also find use in spintronics,” says Dietrich Hesse. This could be a possible future development of electronics, which is why many physicists around the world are researching its basic principles. Spintronics uses both the charge and spin of the electrons to process data with a higher density than is possible in conventional electronics.

In order to advance the multiferroic material sandwich as a spin filter, physicists are first striving to understand precisely how a change of the PZT’s electric polarisation direction affects the magnetic tunnel resistance. Up to now, they only know the details of what happens in the case of the electric polarisation direction that goes hand in hand with the normal tunnel magnetoresistance. “We are unable as yet to explain exactly why the inverted tunnel magnetoresistance appears when the polarisation direction is reversed,” comments Dietrich Hesse. One reason could be the interaction between the ferromagnetic cobalt and the adjoining titanium ions in the PZT. The latter change their position with the polarisation direction. When they get closer to the cobalt layer, they take on their own magnetic momentum on account of the intensive interaction. This magnetic momentum affects the spin direction of the tunnelling electrons.

To explain this connection in detail, Dietrich Hesse and Marin Alexe asked theoretical physicists at the Institute and at the University of Halle for help. They will now calculate the magnetoelectric coupling due to the interaction between the titanium ions of the PZT and the cobalt. However, the help of Dietrich Hesse’s and Marin Alexe’s team is still needed to draw a better comparison between the results of this calculation and the experiments.
They are currently trying to deposit the cobalt cover of their multiferroic material sandwich with a structure that is as regular as that of the other two layers. “Only if we understand exactly how the magnetoelectric coupling works in multiferroic tunnel junctions can we also use it for electronic applications.”


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